期刊
JOURNAL OF HAZARDOUS MATERIALS
卷 340, 期 -, 页码 179-188出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jhazmat.2017.07.011
关键词
Adsorption; Contaminants of emerging concern; Metal-azolate framework; Porous carbon; Pyrolysis
资金
- Kyungpook National University Bokhyeon Research Fund
A series of metal-azolate frameworks or MAFs MAF-4,-5, and -6-were synthesized and pyrolyzed to prepare porous carbons derived from MAFs (CDM-4,-5,-6, respectively). Not only the obtained carbons but also MAFs were characterized and applied for the adsorption of organic contaminants of emerging concern (CECs, including pharmaceuticals and personal care products) such as salicylic acid, clofibric acid, diclofenac sodium, bisphenol-A, and oxybenzone (OXB) from water. CDM-6 was found to be the most remarkable adsorbent among the tested ones (including activated carbon) for all the adsorbates. OXB was taken as a representative adsorbate for detailed adsorption studies as well as understanding the adsorption mechanism. H-bonding (H-acceptor: CDM; H-donor: CECs) was suggested as the principal mechanism for the adsorption of tested adsorbates. Finally, CDMs, especially CDM-6, were suggested as highly efficient and easily recyclable adsorbents for water purification. (C) 2017 Elsevier B.V. All rights reserved.
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