4.2 Article

MnFe2O4 nanoparticles as new catalyst for oxidative degradation of phenol by peroxydisulfate

期刊

JOURNAL OF ENVIRONMENTAL SCIENCES
卷 53, 期 -, 页码 269-277

出版社

SCIENCE PRESS
DOI: 10.1016/j.jes.2015.10.035

关键词

Manganese ferrite; Nanoparticles; Phenol; Peroxydisulfate; Catalytic oxidation

资金

  1. Romanian National Authority for Scientific Research and Innovation, CNCS-UEFISCDI [PN-II-RU-TE-2014-4-0514]

向作者/读者索取更多资源

Manganese ferrite nanopowder was prepared by thermal decomposition at 400 degrees C of the gel synthesized from manganese and iron nitrates and polyvinyl alcohol. X-ray diffractometry evidenced that manganese ferrite was formed as single crystalline phase at this temperature. Scanning electron microscope images evidenced the formation of very fine spherical particles (d < 11 nm) of manganese ferrite, with specific surface area of 147 m(2)/g. The powder obtained at 400 degrees C was used as a catalyst for the oxidative degradation of phenol in aqueous solutions, in the presence of potassium peroxydisulfate as oxidant. High phenol removal efficiencies above 90% were reached at: pH 3-3.5, phenol initial concentration around 50 mg/L, peroxydisulfate: phenol mass ratio 10: 1, and catalyst dose 3 g/L. Total organic carbon measurements showed that the degradation of phenol goes, under these conditions, to mineralization in an extent of 60%. (C) 2016 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.

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