期刊
CHEMICAL SCIENCE
卷 11, 期 3, 页码 791-796出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9sc04498a
关键词
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资金
- Australian Research Council (ARC) Future Fellowship [FT150100479]
- JSPS Postdoctoral Fellowship Program for Foreign Researchers
Generating high surface area mesoporous transition metal boride is interesting because the incorporation of boron atoms generates lattice distortions that lead to the formation of amorphous metal boride with unique properties in catalysis. Here we report the first synthesis of mesoporous cobalt boron amorphous alloy colloidal particles using a soft template-directed assembly approach. Dual reducing agents are used to precisely control the chemical reduction process of mesoporous cobalt boron nanospheres. The Earth-abundance of cobalt boride combined with the high surface area and mesoporous nanoarchitecture enables solar-energy efficient photothermal conversion of CO2 into CO compared to non-porous cobalt boron alloys and commercial cobalt catalysts.
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