期刊
JOURNAL OF MATERIALS CHEMISTRY C
卷 8, 期 3, 页码 1104-1109出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9tc06159b
关键词
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资金
- National Natural Science Foundation of China (NSFC) [61705183, 11875044]
- Nature Science Foundation of Shaanxi Province, China [2019JQ-446]
- Young Talent fund of University Association for Science and Technology in Shaanxi, China [20190113]
- Science Research Foundation of the Education Department of Shaanxi Province, China [19JK0811]
In this work, we investigate VSe2 for generating femtosecond and large energy mode-locked laser pulses for the first time. Two types of VSe2 based saturable absorbers (SAs), microfiber-VSe2 and VSe2/polyvinyl alcohol (PVA), are prepared, which exhibit strong nonlinear optical characteristics with a modulation depth (Delta T) of 22.5% and 1.849%, respectively. In contrast to other transition metal dichalcogenides (TMDCs), theoretical calculations show that VSe2 is a metallic TMDC SA. With the implementation of microfiber-VSe2, conventional soliton mode-locking Er-doped fiber (EDF) laser is demonstrated with an ultrashort pulse duration of 910 fs. Based on VSe2/PVA, a large energy EDF laser is established. The maximum single pulse energy is 25.57 nJ. This study suggests that VSe2 possesses application potential in ultrafast photonics and provides a valuable strategy for the development of TMDC based devices with desirable optoelectronic properties.
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