期刊
ACS APPLIED ENERGY MATERIALS
卷 3, 期 1, 页码 135-140出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsaem.9b01972
关键词
hard carbon; nongraphitizable carbon; negative electrode materials; insertion mechanism; sodium-ion batteries; potassium-ion batteries; rechargeable batteries
资金
- Japan Science and Technology Agency (JST) through SICORP-Concert [JPMJSC17C1]
- MEXT program Elements Strategy Initiative to Form Core Research Center [JPMXP0112101003]
Hard carbon is synthesized by heat-treating macroporous phenolic resin at different temperatures. We study influences of temperature on the structures and electrode properties of the hard carbon in Na and K cells. X-ray diffraction and scattering data of the samples confirm the decreased interlayer distance between sp(2)-carbon sheets and the expanded internal pores at the raised temperatures from 1100 to 1500 degrees C. Reversible capacities in Na cells increase with an increase in the heat-treatment temperature. Hard carbon carbonized at 1500 degrees C delivers the largest capacities of 386 and 336 mAh g(-1) at 10 mA g(-1) in Na and K cells, respectively.
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