期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 22, 期 5, 页码 2648-2659出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cp03638e
关键词
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资金
- Japan Synchrotron Radiation Research Institute (JASRI) [2016B8076, 2017A8005, 2017B8065]
- X-ray Free Electron Laser Utilization Research Project of the Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT)
- X-ray Free Electron Laser Priority Strategy Program of the Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT)
- Proposal Program of SACLA Experimental Instruments of RIKEN
- Japan Society for the Promotion of Science (JSPS) KAKENHI Grant [JP15K17487, JP19H04392]
- Dynamic Alliance for Open Innovation Bridging Human, Environment and Materials'' from the MEXT
- Research Program of Dynamic Alliance for Open Innovation Bridging Human, Environment and Materials'' in Network Joint Research Center for Materials and Devices''
- IMRAM project
- Tohoku University Institute for Promoting Graduate Degree Programs Division for Interdisciplinary Advanced Research and Education
- JSPS KAKENHI [JP19J12870]
- Swedish Research Council
- Swedish Foundation for Strategic Research
- Academy of Finland
Momenta of ions from diiodomethane molecules after multiple ionization by soft-X-ray free-electron-laser pulses are measured. Correlations between the ion momenta are extracted by covariance methods formulated for the use in multiparticle momentum-resolved ion time-of-flight spectroscopy. Femtosecond dynamics of the dissociating multiply charged diiodomethane cations is discussed and interpreted by using simulations based on a classical Coulomb explosion model including charge evolution.
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