期刊
CHEMICAL SCIENCE
卷 11, 期 7, 页码 1912-1917出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9sc04569d
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资金
- TU Braunschweig
Internal alkynes substituted by aliphatic or aromatic moieties or by heteroatoms were converted into sulphur-substituted acrylonitrile derivatives. Key is the use of Pd catalysis, which allows the addition of aromatic and aliphatic thiocyanates in an intra- and intermolecular manner. Substrates with several alkyne units underwent further carbopalladation steps after the initial thiopalladation step, thus generating in a cascade-like fashion an oligoene unit with sulphur at one terminus and the cyano group at the other.
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