4.6 Article

Perovskite Photovoltaics on Roll-To-Roll Coated Ultra-thin Glass as Flexible High-Efficiency Indoor Power Generators

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CELL REPORTS PHYSICAL SCIENCE
卷 1, 期 5, 页码 -

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CELL PRESS
DOI: 10.1016/j.xcrp.2020.100045

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资金

  1. Departamento del Huila's Scholarship Program from Huila, Colombia [677]
  2. Air Force Office of Scientific Research [FA9550-18-1-0233]
  3. European Union's Horizon 2020 research and innovation programme [763989]
  4. Italian Space Agency (ASI) project
  5. PEROSKY-Perovskite and other printable materials for energy application in space [2018-1-R.0]
  6. University of Rome Tor Vergata's Mission: Sustainability'' BiCVision'' project [85-2017-15373]
  7. Italian Ministry of University and Research (MIUR) through the PRIN2017 BOOSTER [2017YXX8AZ]

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The internet of things revolution requires efficient, easy-to-integrate energy harvesting. Here, we report indoor power generation by flexible perovskite solar cells (PSCs) manufactured on roll-to-roll indium-doped tin oxide (ITO)-coated ultra-thin flexible glass (FG) substrates with notable transmittance (>80%), sheet resistance (13 Omega/square), and bendability, surpassing 1,600 bending procedures at 20.5-mm curvature. Optimized PSCs on FG incorporate a mesoporous scaffold over SnO2 compact layers delivering efficiencies of 20.6% (16,7 mu W.cm(-2) power density) and 22.6% (35.0 mu W.cm(-2)) under 200 and 400 lx LED illumination, respectively. These represent, to the best of our knowledge, the highest reported for any indoor flexible solar cell technology, surpassing by a 60%90% margin the prior best-performing flexible PSCs. Specific powers (W/g) delivered by these lightweight cells are 40%-55% higher than their counterparts on polyethylene terephthalate (PET) films and an order of magnitude greater than those on rigid glass, highlighting the potential of flexible FG-PSCs as a key enabling technology for powering indoor electronics of the future.

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