期刊
CHEMICAL COMMUNICATIONS
卷 56, 期 37, 页码 5050-5053出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc01061h
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资金
- Spanish Ministerio de Economia, Industria y Competitividad [CTQ2015-66954-P]
- FEDER/Ministerio de Ciencia, Innovacion y Universidades Agencia Estatal de Investigacion [PGC2018-098660-B-I00]
Substituted 1,3-diazabicyclo[3.1.0]hexanes with two contiguous quaternary stereocentres are readily prepared by catalytic asymmetric [3+2] cycloaddition of alpha-substituted iminoesters with azirines. High diastereoselectivities and enantioselectivities (up to 98% ee) are achieved using Cu-I/(R)-Fesulphos as the catalytic system.
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