期刊
CHEMICAL COMMUNICATIONS
卷 56, 期 39, 页码 5239-5242出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc00608d
关键词
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资金
- National Key Research and Development Program of Ministry of Science and Technology [2017YFB0602201]
- National Natural Science Foundation of China [91945301, 91545203, 21972116, 21872112, 21673188]
- Shaanxi Coal and Chemical Technology Institute Co., Ltd.
Tandem catalysis via methanol intermediate is a promising route for the direct conversion of syngas into aromatics. However, the simultaneous formation of CO2 is a serious problem. Here, we demonstrate that CO2 was formed by the water-gas shift (WGS) reaction (CO + H2O -> CO2 + H-2) over a ZnO-ZrO2/H-ZSM-5 catalyst, and the net CO2 formation could be inhibited without affecting the formation of aromatics by co-feeding CO2.
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