期刊
CRYSTENGCOMM
卷 22, 期 20, 页码 3432-3438出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0ce00435a
关键词
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资金
- National Key Research and Development Program of China [2016YFB0701003]
- National Natural Science Foundation of China [21871248, 21590794]
- K. C. Wong Education Foundation [GJTD-2018-09]
- International Partnership Program of Chinese Academy of Sciences [121522KYSB20190022]
- Key Research Program of Frontier Sciences, CAS [YZDY-SSW-JSC018]
- Jilin Province Science and Technology Development Plan Project [20180101172JC]
- Youth Innovation Promotion Association of Chinese Academy of Sciences [Y2019047]
Bismuth-based nanoparticles, particularly NaBiF4 , have attracted extensive attention as hosts for lanthanides (Ln(3+)) ions and other luminescent ions in recent years. However, the controllable synthesis of NaBiF4 nanoparticles remains a challenge. Herein, different concentrations of Gd3+ ion-doped NaBiF4 : Yb3+/Er(3+ )upconversion nanoparticles (UCNPs) have been successfully synthesized via a facile solvothermal method. By changing the doping levels of Gd3+ ions (0-20%), the size of NaBiF4 : Yb3+/Er3+ UCNPs can be easily tuned from 200 nm to 50 nm, but the nanoparticles always maintained the hexagonal phase structure. Under 980 nm excitation, the as-synthesized NaBiF4 : Yb3+/Er3+/20%Gd3+ UCNPs showed desirable luminescent properties. Furthermore, the 980 nm excited luminescence temperature-sensing behavior of NaBiF4 : Yb3+/Er3+/20%Gd3+ UCNPs was achieved in a wide temperature range from 148 K to 498 K. These results provide strong evidence for the controllable synthesis of NaBiF4 UCNPs and their application in ratiometric temperature sensing.
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