期刊
CHEMICAL SOCIETY REVIEWS
卷 49, 期 12, 页码 3806-3833出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cs00728h
关键词
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资金
- National Natural Science Foundation of China [21776019, 21825501, U1801257]
- National Key Research and Development Program [2016YFA0202500]
- Beijing Natural Science Foundation [L182021]
- Tsinghua University Initiative Scientific Research Program
With the impetus to accelerate worldwide market adoption of electrical vehicles and afford consumer electronics with better user experience, advancing fast-charging technology is an inevitable trend. However, current high-energy lithium-ion batteries are unable to support ultrafast power input without any adverse consequences, with the capacity fade and safety concerns of the mainstream graphite-based anodes being the key technological barrier. The aim of this review is to summarise the fundamentals, challenges, and solutions to enable graphite anodes that are capable of high-rate charging. First, we explore the complicated yet intriguing graphite-electrolyte interface during intercalation based on existing theories. Second, we analyse the key dilemmas facing fast-charging graphite anodes. Finally, some promising strategies proposed during the past few years are highlighted so as to outline current trends and future perspectives in this field.
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