期刊
CHEMICAL COMMUNICATIONS
卷 56, 期 47, 页码 6352-6355出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc02048f
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资金
- National Natural Science Foundation of China [21771144, 21402151]
- Key Laboratory Research Foundation of Education Committee of Shaanxi Province [19JS065]
The dialumane [(L2-AlII)-(AlL2-)-L-II] (L = [(2,6-iPr(2)C(6)H(3))NC(Me)](2); 1) reacts with carbodiimides, RN & xe001;C & xe001;NR (R = Cy, iPr), through insertion, [2+4] cycloaddition, and a hydrogen transfer process. However, with the bulkier carbodiimides (R = dipp = 2,6-iPr(2)C(6)H(3),tBu), the reactions are sterically controlled and lead to the formamidinate products.
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