期刊
JOURNAL OF MATERIALS CHEMISTRY C
卷 8, 期 23, 页码 7812-7819出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0tc01373k
关键词
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资金
- Qingdao University of Technology Staring Foundation [20301721, 20302041]
- Open Research Fund of the State Key Laboratory of Pulsed Power Laser Technology of China in the National University of Defense Technology [SKL2019KF09]
- National Natural Science Foundation of China [U1632151]
PbS quantum dots (QDs) were regarded as promising candidates for photoelectric devices because of their high absorption, multiple exciton generation effect and solution processability. However, their low charge carrier transport behavior impedes their wide application. Here, a ligand exchange process was introduced to fabricate PbS-QD + hybrid perovskite photodetectors. The photodetectors show a high sensitivity, low noise current and high stability under visible to near-infrared light illumination. The devices exhibited an impressive responsivity of similar to 2 x 10(6)A W(-1)and a high photoconductive gain of similar to 3 x 10(6), respectively, with an applied bias of 5 V. Furthermore, the photodetectors display a large detectivity approaching 10(15)Jones and a fast photoresponse up to 1 MHz at room temperature. These great performances suggest that the hybrid perovskite can well passivate the defects of PbS-QDs and provide new insight into the preparation of high-performance nano-devices.
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