期刊
ENERGY & ENVIRONMENTAL SCIENCE
卷 13, 期 8, 页码 2386-2403出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0ee00153h
关键词
-
资金
- National Natural Science Foundation of China [51902150, 51825201]
- Guangdong Basic and Applied Basic Research Foundation [2019A1515110552]
- Key Program of the National Natural Science Foundation of China [51732005]
- National Key Research and Development Program of China [2019YFB1505001]
Solid-state batteries with metallic anodes have attracted great attention due to their high energy density and safety. As an indispensable part of these batteries, solid-state electrolytes (SSEs) with excellent mechanical strength and non-flammability play a significant role in suppressing the growth of dendrites and eliminating the risk of short circuits, whose development could greatly promote the overall battery performance. Recently, metal-organic frameworks (MOFs), a type of porous crystalline inorganic-organic material, have shown potential for the fabrication of high-performance SSEs, which have become an emerging research direction. Benefiting from the rich porosity, controllable functionality and modularity, MOFs not only offer great opportunities for manipulating the physicochemical and electrochemical properties of SSEs, but also provide ideal platforms for investigating the underlying mechanisms of ion conduction and the structure-property relationships. In this perspective, the development of MOF-based SSEs, which include MOF-incorporated polymer hybrids, ionic liquid-laden MOF hybrids, and neat MOFs as SSEs, is outlined. By discussing the pioneering works, both the opportunities and challenges in each SSE category are presented. Additionally, some design principles for MOFs and MOF-based SSEs, as well as the future directions for further development are provided.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据