4.7 Article

Single yttrium sites on carbon-coated TiO2 for efficient electrocatalytic N2 reduction

期刊

CHEMICAL COMMUNICATIONS
卷 56, 期 74, 页码 10910-10913

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc01136c

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资金

  1. National Natural Science Foundation of China [21972010]
  2. Beijing Natural Science Foundation [2192039]
  3. NRF Korea [NRF-2016M3D1A1021147]
  4. DCCEM at the Materials Department, University of Oxford [EP/R010145/1]

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We report single yttrium sites anchored on carbon-coated TiO(2)for efficient and stable electrocatalytic N(2)fixation, delivering an NH(3)faradaic efficiency exceeding 11.0% and an NH(3)yield rate as high as 6.3 mu g(NH3)h(-1)mg(cat.)(-1)at low overpotentials, thus surpassing many reported metal electrocatalysts.

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