期刊
NANOSCALE
卷 12, 期 36, 页码 18497-18522出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0nr04458j
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资金
- Jiangsu Qinglan Project
- Natural Science Foundation of Shandong Province of China [ZR2019BB002]
- Doctoral Fund of QUST [010022873]
- Open Project of Chemistry Department of Qingdao University of Science and Technology [QUSTHX201913]
Developing efficient and low-cost electrocatalysts with unique nanostructures is of great significance for improved electrocatalytic reactions, including the hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and oxygen reduction reaction (ORR). Two-dimensional (2D) metal-organic frameworks (MOFs) have attracted recent attention because of their unique dimension-related properties, such as ultrathin thickness, large specific surface area, and abundant accessible active sites that can act as good precursors for the derivation of a variety of nanocomposites as active materials in electrocatalysis and energy-related devices. In this review, we present recent developments in 2D MOF-derived nanomaterials for hydrogen and oxygen reactions in overall water-splitting and rechargeable Zn-air batteries. The advantages of various synthetic strategies are summarized and discussed in detail. Finally, we discuss the main challenges and future perspectives of the development of 2D MOF-derived electrocatalysts.
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