4.6 Article

Performance modulation of a MgZnO/ZnO heterojunction flexible UV photodetector by the piezophototronic effect

期刊

JOURNAL OF MATERIALS CHEMISTRY C
卷 8, 期 37, 页码 12917-12926

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/d0tc02464c

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资金

  1. National Natural Science Foundation of China [61774023]
  2. Scientific and Technological 13th Five-Year Plan Project of Jilin Provincial Department of Education [JJKH20190587KJ]
  3. Scientific and Technological Development Project of Jilin Province, China [20190101008JH]

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It is essential to modulate materials and their interfaces for excellent device performance. Here, an ultraviolet (UV) photodetector (PD) based on a flexible polyethylene terephthalate (PET)/ZnO/MgZnO heterojunction was successfully fabricated at room temperature. The piezophototronic effect was first used to modulate the transport behavior of the photogenerated carriers at the interface of the MgZnO/ZnO heterojunction. The responsivity increased from 0.23 to 0.95 A W(-1)with the increase in external tensile strain from 0 to 0.18, an increase of similar to 313%. Meanwhile, with the decrease in external compressive strain from 0 to -0.18, the responsivity decreased by similar to 63%. This is owing to the modulation of the junction barrier and photogenerated carrier transport behavior at the MgZnO/ZnO junctions/interfacesviathe piezophototronic effect. Moreover, the PD maintained excellent mechanical stability and reproducibility after different bending cycles 0/50/100/150/200 and excellent environmental stability after storage for over two months, which are beneficial for its practical applications. Furthermore, this study developed a method for modulating the performance of UV PDs, and showed that the piezophototronic effect has important theoretical significance and application prospect for the modulation of heterojunction interfaces.

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