期刊
DIAMOND AND RELATED MATERIALS
卷 109, 期 -, 页码 -出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.diamond.2020.108050
关键词
Carbon nanoparticle; Methane; Flux; Plasma chemical vapor deposition; Thermophoretic force
类别
资金
- JSPS KAKENHI [JP26246036, JP20H00142, JP20J13122]
Carbon nanoparticles (CNPs) were synthesized using Ar + CH4 multi-hollow plasma chemical vapor deposition. The deposition flux of CNPs to a substrate was studied as a function of the plasma discharge time t and the distance L between the plasma and the substrate. CNPs were not deposited for L = 60 and 80 mm, whereas they were deposited for L = 100, 120 and 140 mm. The mean diameter of CNPs was 25 nm irrespective of L. For L = 120 and 140 mm, the flux gradually increased until t = 30 min and then became constant, indicating that thermophoretic force drives CNPs' deposition. Raman spectroscopy showed that a-C:H films were formed for L <= 80 mm, while polymer CNPs were predominant deposits for L >= 100 mm.
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