期刊
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷 45, 期 55, 页码 30009-30016出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2020.08.122
关键词
Geometrical effect; Gliding arc; Methane reforming; Partial oxidation; Pyrolysis
资金
- Technology Development Program to Solve Climate Changes through the National Research Foundation of Korea (NRF) - Ministry of Science, ICT [NRF-2019M1A2A2103681]
Controllability of the kinetic path of methane conversion in plasma driven oxidation reaction is investigated. Different geometries in a rotating gliding arc reactor are adopted to control reaction paths in methane oxidation reaction. Diverging and converging type reactor product different reaction environments in view point of both the reaction time and the degree of thermal activation. In the diverging reactor, the partial oxidation process is dominant with high methane conversion because the diverging section facilitates to elongate the arc length and decrease the flow velocity. Thus, the convective and radiative heat transfer from the arc column to the reactants could be enhanced. The role of plasma in the diverging reactor is mainly igniting and sustaining the partial oxidation, which is rather different from that in the converging reactor where the plasma plays as a heat source for thermal pyrolysis of methane with the help of focusing thermal energy of the arc. (C) 2020 The Author(s). Published by Elsevier Ltd on behalf of Hydrogen Energy Publications LLC.
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