期刊
ADVANCED SCIENCE
卷 7, 期 24, 页码 -出版社
WILEY
DOI: 10.1002/advs.202002368
关键词
extrinsic porosity; metal‐ organic frameworks; molecular sieving; 3D structuring
资金
- Australian Research Council [DE160100569, DP190101864]
- Australian Renewable Energy Agency (ARENA) [2018/RND008]
- European Research Council under the European Union's Horizon 2020 Program (FP/2014-2020)/ERC Grant [771834-POP-CRYSTAL]
- Marie Skodowska-Curie grant [748649-MNEMONIC]
- TU Graz [LP-03]
The structuring of the metal-organic framework material ZIF-8 as films and membranes through the vapor-phase conversion of ZnO fractal nanoparticle networks is reported. The extrinsic porosity of the resulting materials can be tuned from 4% to 66%, and the film thickness can be controlled from 80 nm to 0.23 mm, for areas >100 cm(2). Freestanding and pure metal-organic frameworks (MOF) membranes prepared this way are showcased as separators that minimize capacity fading in model Li-S batteries.
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