期刊
CHEMICAL COMMUNICATIONS
卷 56, 期 92, 页码 14361-14364出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc02206c
关键词
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资金
- National Science Foundation [CHE-1531834, 1551964]
- Virginia Tech National Center for Earth and Environmental Nanotechnology Infrastructure (NanoEarth)
- NSF [ECCS 1542100, ECCS 2025151]
Electrochemical oxidation of 5-hydroxymethylfurfural (HMF) is a promising synthetic route for 2,5-furandicarboxylic acid (FDCA) production. Here, we prepared a nickel(ii)-modified covalent-organic framework (COF) film TpBpy-Ni@FTO for HMF electrooxidation. With a high conversion of HMF (96%), TpBpy-Ni@FTO afforded a 58% FDCA yield. This work underlines the great potential of COF-based materials in electrocatalysis.
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