Formation of nanostructures and optical analogues of massless Dirac particles via femtosecond lasers

Subwavelength-scale surface structures have many important engineering and nanotechnology applications, e.g., superhydrophobicity and light-trapping. However, an effective and economic nanofabrication solution for general engineering materials, e.g., metals or silicon, is still not available to date. In this paper, we present an experimental and theoretical study of the nanostructure formation mechanism based on double time-delayed femtosecond laser beams and the coupled mode theory (CMT), demonstrating the use of an optical analogue of massless Dirac particles for high-throughput nanofabrication for the first time. In the experiments, a variety of complex periodic structures, including hexagonally arranged nanoholes, nano-square array, and periodic ripples, have been fabricated. The formation mechanisms of these nanostructures are explained by the CMT, where a transient plasmonic waveguide array (TPWA) is formed by the interference between the preceding laser and the induced surface plasmon polaritons (SPPs). The SPPs induced by the subsequent laser propagates through the TPWA, resulting in conical diffraction. This result shows the first practical application of the massless Dirac dynamics in nanofabrication. (C) 2020 Optical Society of America under the terms of the OSA Open Access Publishing Agreement