期刊
CRYSTENGCOMM
卷 17, 期 45, 页码 8596-8601出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ce01843a
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资金
- National Research Foundation (NRF), Prime Minister's Office, Singapore under its Campus for Research Excellence and Technological Enterprise (CREATE) Programme-Singapore Peking University Research Centre for a Sustainable Low-Carbon Future
- NTU-A*Star Silicon Technologies Centre of Excellence [11235100003]
- NSFC [21302072, 21201088]
- NSF [BK20130226]
Nitrogen-rich metal-organic framework (N-MOF) nanoparticles with an unusual concave cuboctahedral morphology were prepared through a facile wet-chemical route using benzimidazole as the modulator. Benzimidazole plays an essential role in controlling the concave cuboctahedral morphology of the nanoparticles. By changing the benzimidazole dosage, the resultant morphology can be tuned from a concave octahedron to a concave cuboctahedron. The concave cuboctahedral nanoparticles exhibit high catalytic efficiency for the activation of epoxides with carbon dioxide.
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