期刊
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
卷 8, 期 6, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.jece.2020.104474
关键词
Oil-based drilling cuttings ash; Cr (VI) removal; Contaminated water; Adsorption kinetics; Adsorption mechanism
资金
- Study on Comprehensive Control of Rocky Desertification and Ecological Service Function Improvement in Karst Peaks [2016YFC0502402]
- National Natural Science Foundation of China [51709254]
- Youth Innovation Promotion Association, Chinese Academy of Sciences [2020335]
Secondary pyrolysis oil-based drilling cuttings ash (OBCDA-sp) was employed as a new absorbing material to remove Cr (VI) in wastewater. Varying factors, including pH value, dosage of OBCDA-sp, reaction time and original Cr (VI) contents were studied to investigate the Cr (VI) removal efficiency. Elovich and Pseudo-secondorder models were fitted well with the adsorption kinetics process. In addition, the Langmuir model was well employed to fit Cr (VI) adsorption isotherm on OBCDA-sp. The calculated Cr (VI) theoretic adsorption quantity of OBCDA-sp was 48 mg/g. XPS, SEM-EDS, FTIR and XRD were used to characterize the physicochemical properties of OBDCA-sp. The result shows that the complex process of the Cr (VI) removal involves physical and chemical adsorption, and co-precipitation and reduction. Ba, Fe, S and P element onto OBCDA-sp surface have exerted significant role in Cr (VI) removal.
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