期刊
ORGANIC LETTERS
卷 22, 期 22, 页码 8819-8823出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c03182
关键词
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资金
- National Natural Science Foundation of China [21625203, 21871126, 22001108]
- Jiangxi Educational Committee Foundation of China [GJJ190535]
- Jiangxi Province Science and Technology Project [20202BAB213004]
A novel photocatalytic decarboxylative [2 + 2 + m] cyclization of 1,7-enynes with alkyl N-hydroxyphthalimide (NHP) esters, using tricyclohexylphosphine and potassium iodide as redox catalysts, is reported for the construction of functional polycyclic compounds. This protocol tolerates primary, secondary, and tertiary alkyl NHP esters through a single reaction via decarbonylation, radical addition, C-H functionalization, and cyclization under mild conditions.
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