期刊
NEW JOURNAL OF CHEMISTRY
卷 44, 期 48, 页码 21064-21069出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0nj04548a
关键词
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资金
- Nanjing Tech University [39837146]
- National Natural Science Foundation of China [22001121]
- Natural Science Foundation of Jiangsu Province [BK20180690]
An efficient iron-catalyzed C-O bond functionalization of butyrolactam derivatives with various N-/C-nucleophiles to enable the synthesis of pharmaceutically important butyrolactam derivatives has been developed here. The versatility of the present methodology is demonstrated for direct amination and carbonation by using a variety of sulfonamides, amines, amides, indoles, and 1,3-dicarbonyl compounds under mild conditions. The reaction also showed a wide substrate scope and synthetic simplicity. Additionally, only alcohol was produced as the by-product in all cases.
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