期刊
PHYSICAL REVIEW RESEARCH
卷 2, 期 4, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevResearch.2.042044
关键词
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资金
- Deutsche Forschungsgemeinschaft (DFG) [WU 637/4-1, HO 3324/9-1]
- excellence cluster Munich Center for Quantum Science and Technology (MCQST)
- Alexander von Humboldt foundation
- CREST [JPMJCR15F3]
- JST
Atomistic van der Waals heterostacks are ideal systems for high-temperature exciton condensation because of large exciton binding energies and long lifetimes. Charge transport and electron energy-loss spectroscopy showed first evidence of excitonic many-body states in such two-dimensional materials. Pure optical studies, the most obvious way to access the phase diagram of photogenerated excitons, have been elusive. We observe several criticalities in photogenerated exciton ensembles hosted in MoSe2-WSe2 heterostacks with respect to photoluminescence intensity, linewidth, and temporal coherence pointing towards the transition to a coherent many-body quantum state, consistent with the predicted critical degeneracy temperature. For this state, the estimated occupation is approximately 100% and the phenomena survive above 10 K.Y
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