期刊
FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING
卷 15, 期 4, 页码 -出版社
HIGHER EDUCATION PRESS
DOI: 10.1007/s11783-020-1363-5
关键词
NOx; Chlorobenzene; Simultaneous removal; Kinetic study; Performance prediction; V2O5/TiO2
资金
- National Natural Science Foundation of China [21876093, 21777081]
Research on a V2O5/TiO2 granular catalyst for the simultaneous removal of NO and chlorobenzene showed good synergistic catalytic performance and stability, providing valuable insights for the control of multi-pollutants emission.
The synergetic abatement of multi-pollutants is one of the development trends of flue gas pollution control technology, which is still in the initial stage and facing many challenges. We developed a V2O5/TiO2 granular catalyst and established the kinetic model for the simultaneous removal of NO and chlorobenzene (i.e., an important precursor of dioxins). The granular catalyst synthesized using vanadyl acetylacetonate precursor showed good synergistic catalytic performance and stability. Although the SCR reaction of NO and the oxidation reaction of chlorobenzene mutually inhibited, the reaction order of each reaction was not considerably affected, and the pseudo-first-order reaction kinetics was still followed. The performance prediction of this work is of much value to the understanding and reasonable design of a catalytic system for multi-pollutants (i.e., NO and dioxins) emission control. (c) Higher Education Press 2020
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