4.8 Article

Spectromicroscopy and imaging of photoexcited electron dynamics at in-plane silicon pn junctions

期刊

NANOSCALE
卷 13, 期 4, 页码 2626-2631

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/d0nr07954e

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资金

  1. National Key Research and Development Program of China [2018YFB2200401]
  2. National Natural Science Foundation of China [91950111, 61521004, 11527901, 91850111]

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Theoretically, the kinetic energy of photoelectrons from n-type regions was found to be higher than that of p-type regions due to different work functions. Surprisingly, the outer n-type regions exhibited higher kinetic energy compared to inner n-type regions, caused by reverse bias induced by photoemission. Time-resolved PEEM results showed varying evolution rates of hot electrons in different doping regions.
The ultrafast spatiotemporal imaging of photoexcited electrons is essential to understanding interfacial electron dynamic processes. We used time- and energy-resolved photoemission electron microscopy (PEEM) to investigate the photoexcited electron dynamics at multiplex in-plane silicon pn junctions. We found that the measured kinetic energy of photoelectrons from n-type regions is higher than that from p-type regions owing to different work functions. Interestingly, the kinetic energy of outer n-type regions is higher than that of inner n-type regions, which is caused by the reverse bias induced by photoemission. Time-resolved PEEM results reveal different evolution rates of hot electrons in different doping regions. The rise time of the n-type (outer n-type) regions is faster than that of the p-type (inner n-type) regions. So, closed doping patterns can influence the electron spectra and dynamics at the micro-nano scale. These results help us to understand the ultrafast dynamics of carriers at in-plane interfaces and optimize optoelectronic integrated devices with complex heterojunctions.

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