期刊
NANOSCALE
卷 13, 期 5, 页码 3208-3213出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0nr08758k
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资金
- National Natural Science Foundation of China [21776255, 21972126, 21978264, 21905250]
A flexible method was reported to synthesize Au@Pd core-shell mesoporous nanoflowers with excellent electrocatalytic activity and stability for methanol oxidation reaction. This versatile strategy can be used for the fabrication of core-shell mesoporous nanoflowers with adjustable composition.
The design of bimetallic core-shell nanostructures with mesoporous surfaces is considered significant to strengthen the catalytic activity and stability for direct methanol fuel cells. Here, we report a flexible method to synthesize Au@Pd core-shell mesoporous nanoflowers (Au@mPd NFs) with Au core coated with mesoporous Pd nano-petals, in which polymeric micelle-assembled structures are used as templates to induce the formation of mesopores. Benefiting from the electronic and structural effects, Au@mPd NFs show excellent electrocatalytic activity and stability for methanol oxidation reaction in alkaline electrolytes. This study demonstrates a versatile strategy for the fabrication of core-shell mesoporous nanoflowers with adjustable composition.
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