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An electrochemical perspective on the roles of ligands in the merger of transition-metal catalysis and electrochemistry

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ORGANIC CHEMISTRY FRONTIERS
卷 8, 期 6, 页码 1315-1328

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ROYAL SOC CHEMISTRY
DOI: 10.1039/d0qo01227k

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  1. National Natural Science Foundation of China [21901041]
  2. Fuzhou University [510841]

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The merger of transition-metal catalysis and electrochemistry is a versatile and powerful synthetic tool in organic synthesis, where ligands play crucial roles in fundamental reactions under these combined conditions. Selected transformations enabled by this merger include C-H functionalization, difunctionalization of alkenes, cross-coupling reactions, and carboxylation with CO2.
The merger of transition-metal catalysis and electrochemistry has emerged as a very versatile and robust synthetic tool in organic synthesis. Like in their non-electrochemical variants, ligands also play crucial roles in fundamental reactions in transition-metal catalysis under electrochemical conditions. Herein, a perspective on the roles of ligands in transition-metal catalysis under electrochemical conditions is provided with selected transformations enabled by such a merger including C-H functionalization, difunctionalization of alkenes, cross-coupling reactions and carboxylation with CO2.

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