4.7 Article

Rational design of benzodifuran-functionalized donor-acceptor covalent organic frameworks for photocatalytic hydrogen evolution from water†

期刊

CHEMICAL COMMUNICATIONS
卷 57, 期 36, 页码 4464-4467

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1cc00854d

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资金

  1. National Natural Science Foundation of China [22001153, 21971153, 21772116]
  2. Natural Science Foundation of Shandong Province, China [ZR2020QB036]
  3. Postdoctoral Science Foundation [2020M672118]
  4. Taishan Scholars Program of Shandong Province
  5. Major Basic Research Projects of Shandong Natural Science Foundation [ZR2020ZD32]

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A benzodifuran-based donor-acceptor covalent organic framework was synthesized and utilized for efficient simulated sunlight-driven photocatalytic hydrogen evolution from water, achieving a superior and steady hydrogen evolution rate of 1390 μmol g-1 h-1 and an outstanding apparent quantum yield (AQY) of 7.8% at 420 nm.
A benzodifuran-based donor-acceptor covalent organic framework was synthesized and employed for efficient simulated sunlight-driven photocatalytic hydrogen evolution from water, which exhibited a superior and steady hydrogen evolution rate of 1390 mu mol g(-1) h(-1) and an outstanding apparent quantum yield (AQY) of 7.8% was obtained at 420 nm.

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