期刊
CHEMICAL SOCIETY REVIEWS
卷 50, 期 12, 页码 6914-6949出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cs01134g
关键词
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资金
- AFOSR [FA9550-19-1-0317]
- NSF [DMR 1903990, CMMI 1914713, CBET 1803495, ECCS 1914562]
- Natural Science Foundation of Jiangsu Province in China [BK20201202]
Amorphous inorganic semiconductors have been increasingly studied for their unique properties in various applications such as solar cells and photocatalysis. While their success has been demonstrated, the underlying mechanisms remain unclear. There are promising prospects for further developments in the applications of amorphous inorganic semiconductors.
Amorphous inorganic semiconductors have attracted growing interest due to their unique electrical and optical properties that arise from their intrinsic disordered structure and thermodynamic metastability. Recently, amorphous inorganic semiconductors have been applied in a variety of new technologies, including solar cells, photoelectrocatalysis, and photocatalysis. It has been reported that amorphous phases can improve both efficiency and stability in these applications. While these phenomena are well established, their mechanisms have long remained unclear. This review first introduces the general background of amorphous inorganic semiconductor properties and synthesis. Then, the recent successes and current challenges of amorphous inorganic semiconductor-based materials for applications in solar cells, photoelectrocatalysis, and photocatalysis are addressed. In particular, we discuss the mechanisms behind the remarkable performances of amorphous inorganic semiconductors in these fields. Finally, we provide insightful perspectives into further developments for applications of amorphous inorganic semiconductors.
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