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Recent progress of metal-halide perovskite-based tandem solar cells

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MATERIALS CHEMISTRY FRONTIERS
卷 5, 期 12, 页码 4538-4564

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/d0qm01085e

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资金

  1. Research Grants Council of Hong Kong [15218517, C5037-18G]
  2. Shenzhen Science and Technology Innovation Commission [JCYJ20170413154602102]
  3. funding for Project of Strategic Importance [1-ZE29]
  4. Sir Sze-yuen Chung Endowed Professorship [8-8480]
  5. HK PolyU Postdoctoral Fellowships Scheme [YW3Y]

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This article presents the critical advances of perovskite-based tandem cells, including perovskite-silicon, perovskite-perovskite, perovskite-copper indium gallium selenide, and perovskite-organic TSCs. The paper discusses electrode engineering, interface engineering, bandgap engineering, and processing techniques in detail, while also outlining the future directions and challenges of perovskite TSCs.
Tandem solar cells (TSCs) are devices made of multiple junctions with complementary absorption ranges, aiming to overcome the Shockley-Queisser limit of single-junction solar cells. Currently, metal-halide hybrid perovskite solar cells have risen as an ideal candidate for various tandem cells due to their high open-circuit voltage, tunable optical bandgap, low energy loss, and low-temperature solution processibility. Herein, the critical advances of perovskite-based tandem cells are presented, including perovskite-silicon, perovskite-perovskite, perovskite-copper indium gallium selenide, and perovskite-organic TSCs. Electrode engineering, interface engineering, bandgap engineering, and processing techniques are discussed in detail. The future directions and challenges of perovskite TSCs are also presented.

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