4.6 Article

Tunable solid-state thermal rectification by asymmetric nonlinear radiation

期刊

MATERIALS HORIZONS
卷 8, 期 7, 页码 1998-2005

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1mh00425e

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资金

  1. National Research Foundation of Korea (NRF) - Korea government (MSIT) [2020R1A2C3003199]
  2. National Research Foundation of Korea [2020R1A2C3003199] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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Thermal rectification is achieved using asymmetric nonlinear far-field radiation, allowing tunable solid-state thermal rectification by adjusting asymmetry in thermal conductivity and emissivity. The experiment demonstrated a thermal rectification ratio as high as 93.1%, showing potential applications in heat control and thermal logic gates.
Thermal rectification is a direction-dependent asymmetric heat transport phenomenon. Here we report the tunable solid-state thermal rectification by asymmetric nonlinear far-field radiation. The asymmetry in thermal conductivity and emissivity of a three-terminal device is realized by sputtering a thin metal film (radiation barrier: niobium, copper, or silver) on the top right half of a polyethylene terephthalate strip (emitter). Both the experiment and finite element analysis are in excellent agreement, revealing a thermal rectification ratio (TR) of 13.0% for the niobium-deposited specimen. The simulation demonstrates that the TR can be further increased to 74.5% by tuning asymmetry in thermal conductivity, emissivity, and surface area. The rectification can also be actively controlled, by gating the environmental temperature, resulting in a maximum TR of 93.1%. This work is applicable for a wide range of temperatures and device sizes, which may find applications in on-demand heat control and thermal logic gates.

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