4.6 Article

Active particle diffusion in convection roll arrays

期刊

PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 23, 期 20, 页码 11944-11953

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1cp01088c

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资金

  1. NSF China [11875201, 11935010]
  2. SERB Start-up Research Grant (Young Scientist) [YSS/2014/000853]
  3. UGC-BSR Start-Up Grant [F.30-92/2015]
  4. NTT Research, Army Research Office (ARO) [W911NF-18-1-0358]
  5. Japan Science and Technology Agency (JST) (CREST Grant) [JPMJCR1676]
  6. Japan Society for the Promotion of Science (JSPS) (KAKENHI Grant) [JP20H00134]
  7. Japan Society for the Promotion of Science (JSPS) (JSPS-RFBR) [JPJSBP120194828]
  8. Asian Office of Aerospace Research and Development (AOARD) [FA2386-20-1-4069]
  9. Foundational Questions Institute Fund (FQXi) [FQXi-IAF19-06]

向作者/读者索取更多资源

In this study, the authors numerically investigated the diffusion of active Janus particles in a linear array of planar counter-rotating convection rolls at high Peclet numbers. Active microswimmers exhibit advection-enhanced diffusion, but only for self-propulsion speeds up to a critical value. The diffusion of faster Janus particles is governed by advection along the array's edges, demonstrating distinct diffusion regimes.
Undesired advection effects are unavoidable in most nano-technological applications involving active matter. However, it is conceivable to govern the transport of active particles at the small scales by suitably tuning the relevant advection and self-propulsion parameters. To this purpose, we numerically investigated the Brownian motion of active Janus particles in a linear array of planar counter-rotating convection rolls at high Peclet numbers. Similarly to passive particles, active microswimmers exhibit advection enhanced diffusion, but only for self-propulsion speeds up to a critical value. The diffusion of faster Janus particles is governed by advection along the array's edges, whereby distinct diffusion regimes are observed and characterized. Contrary to passive particles, the relevant spatial distributions of active Janus particles are inhomogeneous. These peculiar properties of active matter are related to the combined action of noise and self-propulsion in a confined geometry and hold regardless of the actual flow boundary conditions.

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