期刊
PHYSICAL REVIEW B
卷 103, 期 16, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.103.L161410
关键词
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资金
- JSPS KAKENHI [JP21H01019, JP18H01154]
- JST CREST [JPMJCR19T1]
The study investigates the spin-dependent optical conductivity of monolayer NbSe2 and finds that pure spin Hall current can be generated under light irradiation, which can be enhanced by electron doping and persists at room temperature. This effect could be utilized in designing opt-spintronics devices based on 2D materials.
Monolayer NbSe2 is a metallic two-dimensional (2D) transition-metal dichalcogenide material. Owing to the lattice structure and the strong atomic spin-orbit coupling (SOC) field, monolayer NbSe2. possesses Ising-type SOC which acts as an effective Zeeman field, leading to the unconventional topological spin properties. In this paper, we numerically calculate spin-dependent optical conductivity of monolayer NbSe2 using Kubo formula based on an effective tight-binding model which includes d(z2), d(x2-y2), and d(xy) orbitals of Nb atoms. Numerical calculation indicates that the up- and down-spin have opposite sign of Hall current, so the pure spin Hall current can be generated in monolayer NbSe2 under light irradiation, owing to the topological nature of monolayer NbSe2, i.e., finite spin Berry curvature. The spin Hall angle is also evaluated. The optically induced spin Hall current can be enhanced by the electron doping and persists even at room temperature. Our results will serve to design opt-spintronics devices such as spin current harvesting by light irradiation on the basis of 2D materials.
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