4.6 Article

Rational design of tandem catalysts using a core-shell structure approach

期刊

NANOSCALE ADVANCES
卷 3, 期 12, 页码 3454-3459

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ROYAL SOC CHEMISTRY
DOI: 10.1039/d1na00310k

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  1. Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany's Excellence Strategy [EXC 2008 - 390540038 - UniSysCat]

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A facile and rational approach was used to synthesize bimetallic heterogeneous tandem catalysts, utilizing core-shell structures to control ensembles of different nanoparticles for chemocatalytic reactions. Successful tandem processes were achieved in CO2 hydrogenation to methane and light olefins.
A facile and rational approach to synthesize bimetallic heterogeneous tandem catalysts is presented. Using core-shell structures, it is possible to create spatially controlled ensembles of different nanoparticles and investigate coupled chemocatalytic reactions. The CO2 hydrogenation to methane and light olefins was tested, achieving a tandem process successfully.

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