4.6 Article

Direct observation of domain wall motion and lattice strain dynamics in ferroelectrics under high-power resonance

期刊

PHYSICAL REVIEW B
卷 103, 期 17, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.103.174113

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资金

  1. Deutsche Forschungsgemeinschaft [414073759, KO 5100/3-1]
  2. Athene Young Investigator program of the TU Darmstadt
  3. Alexander von Humboldt Foundation

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The study measured domain wall motion and lattice strain dynamics of ferroelectrics at resonance using high-power burst excitation and in situ high-energy X-ray diffraction. The research established a general relationship between microstructural strain contributions and macroscopic electromechanical behavior, allowing for the prediction of high-power stability of ferroelectric materials. The results suggest that materials' stability during high-power drive is predominantly related to the basic chemical composition, while piezoelectric hardening mechanisms mainly influence small-signal behavior.
Domain wall motion and lattice strain dynamics of ferroelectrics at resonance were simultaneously measured by combining high-power burst excitation and in situ high-energy x-ray diffraction. The increased loss at high vibration velocity was directly related to the increased domain wall motion, driven by dynamic mechanical stress. A general relationship between the microstructural strain contributions and macroscopic electromechanical behavior was established, allowing the prediction of high-power stability of ferroelectric materials. The results indicate that the materials' stability during high-power drive is predominantly related to the basic chemical composition, while the piezoelectric hardening mechanisms mainly influence the small-signal behavior.

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