期刊
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
卷 9, 期 4, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.jece.2021.105711
关键词
MXene; Dopamine-functionalized; Permeability and selectivity; Long-term stability; Antibacterial ability
资金
- Applied Basic Research Programs of Science and Technology Commission Foundation of Sichuan Province [2021YJ0401]
- Teacher Development Research Start-up Fund of Chengdu University of Technology [109122019KYQD-07276]
In this study, composite membranes were fabricated by modifying MXene materials with PDA, showing improved water flux, dye separation capability, and anti-fouling properties. The modified membrane has potential applications in small molecule separation.
Membrane separation technology has been widely used in the field of industrial dye wastewater treatment. In this work, a series of new composite membranes were fabricated by modifying MXene two-dimensional (2D) materials with polydopamine (PDA) from the mussel biological inspiration via vacuum filtration on cellulose acetate (CA) support. Scanning electron microscope (SEM), transmission electron microscope (TEM), atomic force microscope (AFM), X-ray diffraction technique (XRD), energy spectrum analysis (EDS), have been utilized to evident the successful synthesis of MXene and the modification of MXene by PDA. The resultant PDA@MXene/CA membrane was found to have good hydrophilicity, and the pure water flux reached up to 271.2 L.m(-2).h(-1), which was 277% more than the unmodified membrane. An improvement in dye separation capability has also been noticed using PDA@MXene/CA membranes. The rejection ratio of direct red 28 reached 88.9%, and that of direct black 38 reached 88.6%. Moreover, a strong anti-fouling characteristic with good antibacterial ability of resultant membrane was demonstrated. Therefore, the new modified membrane showed the potential for good application prospects in the field of small molecule separation.
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