期刊
CARBON ENERGY
卷 3, 期 4, 页码 519-540出版社
WILEY
DOI: 10.1002/cey2.127
关键词
methane conversion; methane partial oxidation; methane reforming; photothermal catalysis
类别
资金
- Natural Science Foundation of Jiangsu Province [BK20201345]
- National Natural Science Foundation of China [21707052, 21902009, 21908079]
- Startup Funding at Jiangnan University [1042050205204100, 1045210322190170, 1045281602190010]
- State Key Laboratory of Fine Chemicals, Dalian University of Technology [KF2005]
- Jiangsu Agriculture Science and Technology Innovation Fund [CX(20)3108]
- Fundamental Research Funds for the Central Universities [JUSRP11905, JUSRP52004B]
This review highlights the importance of methane conversion into value-added chemicals, discusses the advanced photothermal synergetic strategy for efficient methane conversion, as well as the methane direct conversion through photocatalysis and thermocatalysis.
Conversion of methane into value-added chemicals is of significance for methane utilization and industrial demand of primary chemical products. The barrier associated with the nonpolar structure of methane and the high bond energy C-H bond (4.57 eV) makes it difficult to realize methane conversion and activation under mild conditions. The photothermal synergetic strategy by combining photon energy and thermo energy provides an advanced philosophy to achieve efficient methane conversion. In this review, we overview the current pioneering studies of photothermal methane indirect conversion and present the methane direct conversion by the way of photocatalysis and thermocatalysis to provide a fundamental understanding of methane activation. Finally, we end this review with a discussion on the remaining challenges and perspectives of methane direct conversion over single-atom catalysts via photothermal synergetic strategy.
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