期刊
NANOSCALE
卷 13, 期 32, 页码 13593-13603出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1nr03409j
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资金
- National Natural Science Foundation of China [21771021, 21822501, 22061130206]
- Beijing Municipal Natural Science Foundation [JQ20003]
- Newton Advanced Fellowship award [NAF\R1\201285]
- Fok Ying-Tong Education Foundation [171008]
- Measurements Fund of Beijing Normal University
- State Key Laboratory of Heavy Oil Processing
This article reviews recent advances in transition metal-based LDHs for photo(electro)chemical water splitting, covering synthesis routes, performance enhancements, and structure-property relationships.
The conversion of solar energy into usable chemical fuels, such as hydrogen gas, via photo(electro)chemical water splitting is a promising approach for creating a carbon neutral energy ecosystem. The deployment of this technology industrially and at scale requires photoelectrodes that are highly active, cost-effective, and stable. To create these new photoelectrodes, transition metal-based electrocatalysts have been proposed as potential cocatalysts for improving the performance of water splitting catalysts. Layered double hydroxides (LDHs) are a class of clays with brucite like layers and intercalated anions. Transition metal-based LDHs are increasingly popular in the field of photo(electro)chemical water splitting due to their unique physicochemical properties. This article aims to review recent advances in transition metal-based LDHs for photo(electro)chemical water splitting. This article provides a brief overview of the research in a format approachable for the general scientific audience. Specifically, this review examines the following areas: (i) routes for synthesis of transition metal-based LDHs, (ii) recent developments in transition metal-based LDHs for photo(electro)chemical water splitting, and (iii) an overview of the structure-property relationships therein.
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