4.8 Article

Sustainable off-grid desalination of hypersaline waters using Janus wood evaporators

期刊

ENERGY & ENVIRONMENTAL SCIENCE
卷 14, 期 10, 页码 5347-5357

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1ee01505b

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资金

  1. Princeton Center for Complex Materials (PCCM)
  2. National Science Foundation (NSF)-MRSEC program [DMR-2011750]
  3. Princeton Catalysis Initiative (PCI)
  4. Materials Research Science and Engineering Center (MRSEC), National Science Foundation (NSF) [DMR-1420541]

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A sustainable Janus wood evaporator has been developed to address the challenges of salt accumulation on solar absorbers in solar-thermal evaporation, achieving high evaporation efficiencies in hypersaline water. This evaporator features asymmetric surface wettability with hydrophobic and hydrophilic layers, showcasing persistent salt-resistance and superior thermal insulation. A life cycle assessment suggests that the Janus wood evaporator offers a functional and more sustainable option for off-grid desalination and humanitarian efforts.
Solar-thermal evaporation is a promising technology for energy-efficient desalination, but salt accumulation on solar absorbers and system longevity are the major challenges that hinder its widespread application. In this study, we present a sustainable Janus wood evaporator that overcomes these challenges and achieves a record-high evaporation efficiencies in hypersaline water, one of the most difficult water sources to treat via desalination. The Janus wood evaporator has asymmetric surface wettability, where the top layer acts as a hydrophobic solar absorber with water blockage and salt resistance, while the bottom hydrophilic wood layer allows for rapid water replenishment and superior thermal insulation. An evaporation efficiency of 82.0% is achieved for 20% NaCl solution under 1 sun, and persistent salt-resistance is observed during a 10-cycle long-term test. To ensure the environmental impact of the Janus wood evaporator, for the first time, a life cycle assessment (LCA) is conducted to compare this Janus wood evaporator with the emerging Janus evaporators, indicating a functional and more sustainable opportunity for off-grid desalination and humanitarian efforts.

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