4.6 Article

Light-matter coupling and quantum geometry in moire materials

期刊

PHYSICAL REVIEW B
卷 104, 期 6, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.104.064306

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资金

  1. Academy of Finland [303351, 307419, 327293]
  2. DFG Emmy Noether program [SE 2558/2]
  3. Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) [RTG 1995, SPP 2244, EXC2004/1-390534769]
  4. Max Planck-New York City Center for Non-Equilibrium Quantum Phenomena

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Quantum geometry plays a crucial role in the light-matter coupling of flat-band and moire materials, making strong light-matter coupling more achievable by suppressing the electronic kinetic energy. Despite the nearly vanishing band velocities and curvatures, light can still couple to flat bands through geometric contributions. The study provides fundamental principles and tools for controlling emergent electronic properties in flat-band and moire materials based on light-matter coupling.
Quantum geometry has been identified as an important ingredient for the physics of quantum materials and especially of flat-band systems, such as moire materials. On the other hand, the coupling between light and matter is of key importance across disciplines and especially for Floquet and cavity engineering of solids. Here we present fundamental relations between light-matter coupling and quantum geometry of Bloch wave functions, with a particular focus on flat-band and moire materials, in which the quenching of the electronic kinetic energy could allow one to reach the limit of strong light-matter coupling more easily than in highly dispersive systems. We show that, despite the fact that flat bands have vanishing band velocities and curvatures, light couples to them via geometric contributions. Specifically, the intraband quantum metric allows diamagnetic coupling inside a flat band; the interband Berry connection governs dipole matrix elements between flat and dispersive bands. We illustrate these effects in two representative model systems: (i) a sawtooth quantum chain with a single flat band and (ii) a tight-binding model for twisted bilayer graphene. For (i) we highlight the importance of quantum geometry by demonstrating a nonvanishing diamagnetic light-matter coupling inside the flat band. For (ii) we explore the twist-angle dependence of various light-matter coupling matrix elements. Furthermore, at the magic angle corresponding to almost flat bands, we show a Floquet-topological gap opening under irradiation with circularly polarized light despite the nearly vanishing Fermi velocity. We discuss how these findings provide fundamental design principles and tools for light-matter-coupling-based control of emergent electronic properties in flat-band and moire materials.

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