A bioinspired porous-designed hydrogel@polyurethane sponge piezoresistive sensor for human-machine interfacing

Conductive coating sponge piezoresistive pressure sensors are attracting much attention because of their simple production and convenient signal acquisition. However, manufacturing sponge-structure pressure-sensing materials with high compressibility and wide pressure detection ranges is difficult because of the instability of rigid and brittle conductive coatings at large strains. Herein, a tough conductive hydrogel@polyurethane (PU) sponge with a porous design is prepared via immersion of a polyurethane sponge in a low-cost and biocompatible polyvinyl alcohol (PVA)/glycerin (Gl)/sodium chloride (NaCl) solution. The sensor based on the hydrogel/elastomer sponge composite material exhibits a compressible range of 0-93%, a pressure detection range of 100 Pa-470.2 kPa, and 10 000-cycle stability (80% strain) because of the compressibility, flexibility, and toughness of the porous hydrogel coating. Benefiting from the resistance change mechanism of microporous compression, the sensor also exhibits a wide range of linear resistance changes, and the corresponding sensitivity and gauge factor (GF) are -0.083 kPa(--) (100 Pa-10.0 kPa) and -1.33 (1-60% strain), respectively. Based on its flexibility, compressibility, and wide-ranging linear resistance changes, the proposed sensor has huge potential application in human activity monitoring, electronic skin, and wearable electronic devices.

Automated summary

A conductive hydrogel@polyurethane (PU) sponge with high compressibility and wide pressure detection range was successfully prepared in this study. The sensor based on the porous hydrogel coating exhibited excellent performance due to its compressibility, flexibility, and toughness.