4.6 Article

Application of high-efficiency green fluorescent carbon dots prepared by acid catalysis in multicolour LEDs

期刊

RSC ADVANCES
卷 11, 期 60, 页码 38033-38039

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ROYAL SOC CHEMISTRY
DOI: 10.1039/d1ra07280c

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资金

  1. National Natural Science Foundation [21961036]
  2. China Agriculture Research System [CARS-21]
  3. Applied Basic Research Programs of Science and Technology Department of Yunnan Province [202101AT070041, 202002AA10007, 202102AE090042, 2019ZG0901]
  4. Key Laboratory of State Forestry Administration for Highly-Efficient Utilization of Forestry Biomass Resources in Southwest China [2019-KF05]

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In this study, efficient green fluorescent carbon dots were prepared using acid catalysts, and the mechanism of acid-catalyzed fluorescence redshift and improved quantum yield of CDs was discussed. By manipulating the fluorescence tunability of CDs, LED emitting different spectra with excellent performance were successfully prepared.
Acidic reagents play an important role in the preparation of carbon dots (CDs). Therefore, we prepared efficient green fluorescent CDs by potassium bisulfate, acetic acid and hydrochloric acid catalysis and discussed why the acid catalyst induced a fluorescence redshift and improved the quantum yield of the CDs. Furthermore, the concentration-dependent photoluminescence behaviour of the CDs was characterized. CD/PVA composites emitting green to yellow light were obtained by exploiting the fluorescence tunability of CDs. Based on different light-emitting diode substrates, green, yellow and white light-emitting diodes with excellent performance were prepared.

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