期刊
DESALINATION AND WATER TREATMENT
卷 241, 期 -, 页码 135-145出版社
DESALINATION PUBL
DOI: 10.5004/dwt.2021.27824
关键词
Photocatalytic; FeNi3; SiO2; TiO2; Solar light; Humic acid; Degradation efficiency; By-products
资金
- [455617]
The study evaluated the degradation ability of FeNi3/SiO2/TiO2 magnetic nanocomposite for degrading humic acid, demonstrating efficient and eco-friendly degradation with a degradation efficiency of 89% under optimal conditions. The interaction between FeNi3/SiO2/TiO2 and LED solar light effectively degraded humic acid, and the catalyst can be recycled six times with minimal degradation capacity loss.
The present study evaluates the degradation ability of FeNi3/SiO2/TiO2 magnetic nanocomposite as a catalyst for degrading humic acid molecules in a photocatalytic process using simulated solar light-induced by light-emitting diode (LED) illumination. The morphology and structural properties of the used catalyst and the physiochemical factors influencing humic acid degradation (solution pH, catalyst dose, humic acid concentration, and reaction time) were examined in detail. In addition, the kinetics reaction type and mechanism of humic acid degradation were studied. Results showed that the suggested treatment method was efficient during the degradation of humic acid molecules, with non-toxic chemicals generated at the end of degradation, namely carbon dioxide and water. In addition, a degradation efficiency of 89% was achieved under optimal conditions. Compared with other similar methods, this study demonstrated that the interaction between FeNi3/SiO2/TiO2 and LED solar light effectively degraded humic acid in an eco-friendly manner. The degradation reaction kinetics can be mathematically represented by a pseudo-first-order formula. The used catalyst can be recycled in the suggested treatment system six times with negligible losses in its degradation capacity. This study is necessary to understand how photocatalytic wastewater purification of humic acid.
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