期刊
JOURNAL OF MATERIALS CHEMISTRY C
卷 9, 期 34, 页码 11085-11090出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1tc03331j
关键词
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资金
- National Key Research and Development Program of China [2018YFA0704403]
- NSFC [62074064]
- Innovation Fund of WNLO
2D layered perovskites have been demonstrated as excellent candidate materials for narrowband photodetectors, and researchers have successfully fabricated narrowband photodetector arrays based on this material for imaging. The prepared photodetector exhibits a narrow photo-response peak and high external quantum efficiency.
Narrowband photodetectors, which are capable of detecting light within a narrow spectral range, have important applications in the fields of digital cameras, biosensing and artificial vision. In particular, 2D layered perovskites stand out as good candidate materials for narrowband photodetectors due to their prominent properties, such as natural quantum-well structure and tunable bandgap. Although narrowband photodetectors based on 2D perovskites have been presented recently, for some practical applications, including optical communication and imaging, narrowband photodetector arrays need to be prepared, which has not been reported yet. Here, we have demonstrated the fabrication of 12 x 11 narrowband photodetector arrays based on 2D (BA)(2)PbI4 perovskites to realize imaging for the first time. The as-prepared photodetector exhibits a narrow photo-response peak centered at around 546 nm with a full width at half maximum of 24 nm. Besides, it shows a high external quantum efficiency of 350% and a detectivity of 2.17 x 10(11) Jones under 546 nm illumination. Furthermore, the narrowband photodetector arrays can also realize imaging under monochromatic light illumination from the back side of the device with wavelength selection.
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