期刊
ENERGY & ENVIRONMENTAL SCIENCE
卷 10, 期 4, 页码 860-884出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ee03499c
关键词
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资金
- ALCA Project of JST, Japan
- National Basic Research Program of China [2014CB932300]
- National Natural Science Foundation (NSF) of China [21633003, 21373111]
Li-air batteries have drawn considerable attention due to their high energy density and promising implementation in long-range electric vehicle and wearable electronic devices. Nevertheless, safety concerns, mainly derived from the use of flammable organic liquid electrolytes, have become a major bottleneck to the strategically crucial applications of Li-air batteries. Polymer electrolytes with non-toxicity, low vapor pressure, and non-flammable properties provide a feasible solution to safety issues through the replacement of organic liquid electrolytes, although fundamental understanding of polymer electrolytes for Li-air batteries is still insufficient. Accordingly, substantial research efforts have been devoted to achieving next-generation solid-state Li-air batteries with polymer electrolytes. Herein, we provide a specific review on the development of polymer electrolytes for Li-O-2 (air) batteries, from comprehensive insight to emerging horizons, especially in understanding the underpinning chemistry and electrochemistry that govern the properties of polymer electrolytes for the solid-state lithium-air batteries. The discussion will highlight the recent progress in and challenges associated with polymer electrolytes for Li-O-2 (air) batteries, as well as corresponding strategic perspectives.
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